This is the list I submitted (alas, no time for pictures!):
1. Cabaret
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2. The Red Shoes
3. Brief Encounter
4. Sunrise: A Song of Two Humans
5. A Letter to Three Wives
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6. My Neighbour Totoro
7. Casablanca
8. In America
9. Three Colours: Blue
10. Singin' in the Rain
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11. Eureka
12. The Seventh Seal
13. It Happened One Night
14. Les roseaux sauvages (Wild Reeds)
15. The Lion in Winter (1968)
16. Before Sunrise
17. M
18. Once Upon a Time in the West
19. It's a Wonderful Life
20. A Matter of Life and Death
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21. Grave of the Fireflies
22. The Philadelphia Story
23. Die Abenteuer des Prinzen Achmed (The Adventures of Prince Achmed)
24. The Adventures of Robin Hood
25. Der Himmel über Berlin (Wings of Desire)
26. All About My Mother
27. The Station Agent
28. Aguirre, der Zorn Gottes
29. Sunset Blvd.
30. Four Weddings and a Funeral
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31. Three Colours: Red
32. Vertigo
33. My Own Private Idaho
34. Dial M for Murder
35. Annie Hall
36. Breathless
37. The Night of the Hunter
38. Scenes From a Marriage
39. Mary Poppins
40. Volver
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41. The Life and Death of Colonel Blimp
42. Rebecca
43. The Thief of Bagdad
44. In the Mood for Love
45. An American in Paris
46. Days of Heaven
47. In a Lonely Place
48. To be or not to be
49. In the Bedroom
50. Don't Look Now
51. The 39 Steps
52. A Fish Called Wanda
53. Who's Afraid of Virginia Woolf?
54. Sissi
55. The Matrix
56. Groundhog Day
57. La Double Vie de Véronique
58. Blade Runner
59. The Remains of the Day
60. The Fisher King
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61. Persona
62. The Good, The Bad and The Ugly
63. The Shop Around the Corner
64. Edward Scissorhands
65. Bright Star
66. Titus
67. 4 Months, 3 Weeks and 2 Days
68. City Lights
69. Rosencrantz and Guildenstern are Dead
70. The Purple Rose of Cairo
71. The Fall
72. Much Ado About Nothing
73. The Sweet Hereafter
74. Eyes Wide Shut
75. Dr. Strangelove or: How I Learned to Stop Worrying and Love the Bomb
76. Synecdoche, New York
77. Rio Bravo
78. Bridget Jones's Diary
79. Psycho
80. Paris, Texas
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81. McCabe and Mrs Miller
82. Mulholland Dr.
83. Shame (2011)
84. Happy Together
85. Badlands
86. Howl' Moving Castle
87. Holiday
88. Moonrise Kingdom
89. Crouching Tiger, Hidden Dragon
90. Ordinary People
91. Rope
92. Metropolis (1927)
93. Eat, Drink, Man, Woman
94. Requiem for a Dream
95. The Piano
96. Spring, Summer, Fall, Winter ... and Spring
97. All About Eve
98. Das weisse Band (The White Ribbon)
99. YiYi
100. Witness for the Prosecution
These films were cut from my previous list:
North by Northwest
A Serious Man
Winter Light
Beauty and the Beast
Eternal Sunshine Of The Spotless Mind
Magnolia
Central Station
Laura
The Ice Storm
These are my new additions:
Vertigo
Scenes from a Marriage
In a Lonely Place
Rio Bravo
The Fall
Ordinary People
Shame
Moonrise Kingdom
Much Ado About Nothing